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Stone after being mesmerised by his performance in Bicho de Sete Cabeças.Since Santoro did not have an agent in North America, Ackerman contacted Santoro's father.Santoro went on to play parts in many of Globo's telenovelas, such as Olho no Olho (1993), Pátria Minha (1994), Explode Coração (1995), O Amor Está no Ar (1997), Suave Veneno (1999) and Mulheres Apaixonadas (2003), as well as the miniseries Hilda Furacão (1998), in the role of a priest.Santoro was also the voice actor of the titular character in Stuart Little and its sequel in the Brazilian dubbed copies.
By the end of the film, he received a standing ovation from the audience.
He also went on to win the festival's best actor trophy.
After Bicho, his reputation as an actor had been solidified and he was cast as the male lead in Abril Despedaçado (Behind the Sun), one of the nominees for best foreign film in the 2002 Golden Globe Awards.
He spent two months filming in Rome, alongside renowned actors such as Helen Mirren and Anne Bancroft. Stone, he received an offer from Columbia Pictures for a part in the blockbuster Charlie's Angels: Full Throttle.
His performance in Charlie's Angels kick-started his career in Hollywood.
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In 2006, Santoro joined the cast of Lost as survivor of Oceanic Flight 815, Paulo.